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Abstract In contrast to surface greenhouse warming, surface greenhouse cooling has been less explored, especially on multi-century timescales. Here, we assess the processes controlling the pacing and magnitude of the multi-century surface temperature response to instantaneously doubling and halving atmospheric carbon dioxide concentrations in a modern global coupled climate model. Over the first decades, surface greenhouse warming is larger and faster than surface greenhouse cooling both globally and at high northern latitudes (45–90° N). Yet, this initial multi-decadal response difference does not persist. After year 150, additional surface warming is negligible, but surface cooling and sea ice expansion continues. Notably, the equilibration timescale for high northern latitude surface cooling (∼437 years) is more than double the equivalent timescale for warming. The high northern latitude responses differ most at the sea ice edge. Under greenhouse cooling, the sea ice edge slowly creeps southward into the mid-latitude oceans amplified by positive lapse rate and surface albedo feedbacks. While greenhouse warming and sea ice loss at high northern latitudes occurs on multi-decadal timescales, greenhouse cooling and sea ice expansion occurs on multi-century timescales. Overall, this work shows the importance of multi-century timescales and sea ice processes for understanding high northern latitude climate responses. 

Abstract Arctic amplification (AA), referring to the phenomenon of amplified warming in the Arctic compared to the warming in the rest of the globe, is generally attributed to the increasing concentrations of carbon dioxide (CO₂) in the atmosphere. However, little attention has been paid to the mechanisms and quantitative variations of AA under decreasing levels of CO₂, when cooling where the Arctic region is considerably larger than over the rest of the planet. Analyzing climate model experiments forced with a wide range of CO₂concentrations (from 1/8× to 8×CO₂, with respect to preindustrial levels), we show that AA indeed occurs under decreasing CO₂concentrations, and it is stronger than AA under increasing CO₂concentrations. Feedback analysis reveals that the Planck, lapse-rate, and albedo feedbacks are the main contributors to producing AAs forced by CO₂increase and decrease, but the stronger lapse-rate feedback associated with decreasing CO₂level gives rise to stronger AA. We further find that the increasing CO₂concentrations delay the peak month of AA from November to December or January, depending on the forcing strength. In contrast, decreasing CO₂levels cannot shift the peak of AA earlier than October, as a consequence of the maximum sea-ice increase in September which is independent of forcing strength. Such seasonality changes are also presented in the lapse-rate feedback, but do not appear in other feedbacks nor in the atmospheric and oceanic heat transport processeses. Our results highlight the strongly asymmetric responses of AA, as evidenced by the different changes in its intensity and seasonality, to the increasing and decreasing CO₂concentrations. These findings have significant implications for understanding how carbon removal could impact the Arctic climate, ecosystems, and socio-economic activities.